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The La Liga champions were favorites to secure the defender's signing in March, but they were late in the race after PSG offered better conditions.
Juventus, Manchester United and Liverpool are among other European giants in pursuit of the Dutch international, who played a key role in Ajax 's national double triumph and qualified for the semifinals of the Champions League in 2018/19.
ESPN FC said Barca would turn to Mino Raiola, De Ligt's representative, this week as he tried to beat PSG at the center post.
It is unclear whether the Spanish club will be willing to improve conditions it had previously offered the Dutch.
Barcelona has already entered into an agreement with Ajax to sign the player for around 80 million euros when it accepts personal conditions.
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